Repozytorium

Structure and properties of a new rigid tripodal oxime ligand.

Autorzy

Dejan Premužić

Aleksander Filarowski

Małgorzata Hołyńska

Rok wydania

2017

Czasopismo

Journal of Molecular Structure

Numer woluminu

1136

Strony

100-106

DOI

10.1016/j.molstruc.2017.01.087

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Synthesis and properties of a new rigid tripodal oxime ligand are reported. The ligand is a derivative of phloroglucine with three carboxime arms alternate with hydroxyl groups and three intramolecular Osingle bondH⋯N hydrogen bonds. Intermolecular Osingle bondH⋯O hydrogen bonds result in formation of a characteristic three-dimensional network. The structure of the compound is further analyzed and confirmed by NMR, IR and MS-techniques. DFT calculations were employed to accomplish the analysis of both the hydrogen bonding and the conformational state of the ligand under study. Additionally, the study addresses the way the conformational state and metal-replacement influence the tautomeric equilibrium OH⋯N ⇆ O−⋯+HN in the studied moieties.

Słowa kluczowe

single crystal structure analysis, hydrogen bonding, Oxime ligands, density functional calculations

Adres publiczny

http://dx.doi.org/10.1016/j.molstruc.2017.01.087

Strona internetowa wydawcy

http://www.elsevier.com

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