Repozytorium

Structure and spectroscopy of NaNd(SP)4chelate: a new type of lanthanide luminophore.

Autorzy

Dagmara Kulesza

Marcin Sobczyk

Janina Legendziewicz

O. M. Moroz

Vladimir M. Amirkhanov

Rok wydania

2010

Czasopismo

Structural Chemistry

Numer woluminu

21

Strony

425-438

DOI

10.1007/s11224-009-9548-3

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Lanthanideb-diketones and their derivativesare extensively studied coordination compounds, due totheir luminescent properties and many possible applica-tions. The tetrakisNd(III) complex with phosphorylatedsulfonylamides derivatives ofb-diketones was synthe-sized. The X-ray diffraction showed that the compound offormula {[Na[Ln(SP)4]}n(SP=C6H5S(O)2NP(O)(OCH3)2;Ln=Nd(III) crystallize in the monoclinic P21/c spacegroup with the following unit-cell parameters:a=22.006(4)A,b=11.075(2)A,c=22.334(5)A, andb=118.71(3)°. The molecular structure of the investigatedcompound is polymeric. The lanthanide ions as well as thesodium ions are coordinated by sulfonyl and phosphorylgroups of the ligand, and because of the bridging behavior,link different units of the polymer. High-resolutionabsorption, emission, and excitation spectra of neodymiumcrystals were measured at 298, 77, and 4K temperatures.

Słowa kluczowe

Neodymium ion, crystal structure, spectroscopy, Intensity parameters, crystal field analysis, absorption and emission spectra

Adres publiczny

http://dx.doi.org/10.1007/s11224-009-9548-3

Strona internetowa wydawcy

http://link.springer.com

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