Repozytorium

Structural and magnetic studies of tetranuclear heterometallic M/Cr (M=Co, Mn) complexes self-assembled from zerovalent cobalt or manganese, Reineckes salt and diethanolamine.

Autorzy

V. V. Semenaka

Oksana V. Nesterova

Vladimir N. Kokozay

R. I. Zybatyuk

Oleg V. Shishkin

Roman Boča

Carlos J. Gómez-García

J. M. Clemente-Juan

Julia Jezierska

Rok wydania

2010

Czasopismo

Polyhedron

Numer woluminu

29

Strony

1326-1336

DOI

10.1016/j.poly.2009.12.032

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Four novel heterometallic complexes [Co2Cr2(NCS)4(HDea)2(Dea)2]·4dmf (1), [Co2Cr2(NCS)4(HDea)2(Dea)2]·4dmso (2), [Mn2Cr2(NCS)4(HDea)2(Dea)2(dmf)2]·2dmf (3) and [Mn2Cr2(NCS)4(HDea)2(Dea)2(dmso)2]·4dmso (4) have been prepared using zerovalent cobalt (1, 2) or manganese (3, 4), Reineckes salt, ammonium thiocyanate and a non-aqueous solution of diethanolamine (H2Dea) in air. The single X-ray analysis reveals that all compounds have similar centrosymmetric crystal structures based on a tetranuclear {M2Cr23-O)2(μ-O)4} (M = Co, Mn) core. Variable-temperature magnetic susceptibility measurements of 1, 2 and 4 show antiferromagnetic coupling between the magnetic centers, while 3 exhibits a ferromagnetic behavior.

Słowa kluczowe

Heterometallic complexes, Diethanolamine, Magnetism

Adres publiczny

https://doi.org/10.1016/j.poly.2009.12.032

Strona internetowa wydawcy

http://www.elsevier.com

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