Repozytorium

Implementation and validation of a multi-purpose virtual spectrometer for large systems in complex environments

Autorzy

Vincenzo Barone

Alberto Baiardi

Małgorzata Biczysko

Julien Bloino

Chiara Cappelli

Filippo Lipparini

Rok wydania

2012

Czasopismo

Physical Chemistry Chemical Physics

Numer woluminu

14

Strony

12404-12422

DOI

10.1039/c2cp41006k

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Despite impressive advances of computational spectroscopy, a robust and user-friendly multi-frequency virtual spectrometer is not yet available. This contribution summarises ongoing efforts in our research group toward the implementation and validation of such a tool with special reference to the building blocks of biomolecules in their natural environment. Our integrated computational tool allows the computation of several kinds of spectra, including vibrational (e.g. IR, VCD), electronic (e.g. absorption, emission, ECD) as well as magnetic resonance (e.g. ESR, NMR) for both closed- and open-shell systems in vacuo and in condensed phases, and includes facilities for drawing, comparing, and modifying all the computed spectra. A number of test cases involving a combination of different spectroscopic ranges will be discussed in order to point out strengths, limitations, and ongoing developments of our research plan.

Adres publiczny

http://dx.doi.org/10.1039/c2cp41006k

Strona internetowa wydawcy

https://www.rsc.org/

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