Repozytorium

Magnetic Properties of Nitroxide Spin Probes: Reliable Account of Molecular Motions and Nonspecific Solvent Effects by Time-Dependent and Time-Independent Approaches

Autorzy

Michele Pavone

Małgorzata Biczysko

Nadia Rega

Vincenzo Barone

Rok wydania

2010

Czasopismo

Journal of Physical Chemistry B

Numer woluminu

114

Strony

11509-11514

DOI

10.1021/jp102232c

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Application of a new integrated computational approach for two widely used nitroxide spin probes allows to show unequivocally that proper account of stereoelectronic, environmental, and dynamical effects leads to magnetic properties in quantitative agreement with experimental results without the need of any empirical parameter. Together with their specific interest, our results point out, in our opinion, the importance of developing and validating computational approaches able to switch on and off different effects, including environmental and dynamical ones, in order to evaluate their specific role in determining the overall experimental outcome.

Adres publiczny

http://dx.doi.org/10.1021/jp102232c

Strona internetowa wydawcy

https://www.acs.org/content/acs/en.html

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