Repozytorium

The Cu2+binding properties of branched peptides based on L-2,3-diaminopropionic acid.

Autorzy

Łukasz Szyrwiel

Łukasz Szczukowski

József Sándor Pap

Bartosz Setner

Zbigniew Szewczuk

Wiesław Malinka

Rok wydania

2014

Czasopismo

Inorganic Chemistry

Numer woluminu

53

Strony

7951-7959

DOI

10.1021/ic5007428

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Three new branched peptides, namely, H-Gly-Dap(H-Gly)-Gly-NH2 (3G), H-His-Dap(H-His)-Gly-NH2 (2HG), and H-Gly-Dap(H-Gly)-His-NH2 (2GH), where Dap stands for the 2,3-diaminopropionic acid residue, were synthesized by solid phase procedures. Because of the junction at Dap these peptides have three available pending arms for metal chelation. The complex formation between these peptides and 1 equiv of Cu2+ was investigated as a function of pH by potentiometry ultraviolet–visible absorption, circular dichroism, and X-band electron paramagnetic resonance spectroscopy in aqueous medium. Our results clearly demonstrate that cooperation between all three peptide arms essentially contributes to the stability of copper(II) complexes.

Adres publiczny

http://dx.doi.org/10.1021/ic5007428

Strona internetowa wydawcy

https://www.acs.org/content/acs/en.html

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