Repozytorium

Structure-activity relationship disturbed by a solvolytic process: study on the [Cu(II)-4-nitropyridine N-oxide derivative] system.

Autorzy

Aniela Puszko

Andrzej Kochel

Joanna Wietrzyk

Beata Filip-Psurska

Julia Jezierska

Mariola Puszyńska-Tuszkanow

Zbigniew Staszak

Anna Adach

Jadwiga Lorenc

Maria Cieślak-Golonka

Rok wydania

2013

Czasopismo

Polyhedron

Numer woluminu

50

Strony

146-153

DOI

10.1016/j.poly.2012.09.060

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The chelate complex [CuCl2(L)] where L = 2-methylamino-3-methyl-4-nitropyridine-N-oxide has been obtained and characterized, both physicochemically (by the X-ray structure analysis of the complex and the ligand, FTIR, EPR and electronic spectroscopy, and thermal analysis) and cytotoxically (MCF-7, A549, SW707, P388, Balb3T3). In solution, atypically for chelate complexes, it undergoes rapid solvolysis forming various 6- (or 5) and 4-coordinate species, depending upon the solvent. Such rapid decomposition may indicate a catalytic effect of the copper operating in the system. However, the cytotoxic activity in solution for the new copper chelate complex appeared to be a surprisingly low. Thus, before drawing any conclusions on the structure–activity relationship, one must carefully check the chemical identity of the compound(s) in both phases.

Słowa kluczowe

Copper(II) complexes, 4-Nitropyridine-N-oxide derivative, Crystal structure, Solvolisis

Adres publiczny

http://dx.doi.org/10.1016/j.poly.2012.09.060

Strona internetowa wydawcy

http://www.elsevier.com

Podobne publikacje
2011

Systematic coordination chemistry and cytotoxicity of copper(II) complexes with methyl substituted 4-nitropyridine N-oxides.

Puszko Aniela, Brzuszkiewicz Anna, Jezierska Julia, Adach Anna, Wietrzyk Joanna, Filip B., Pełczyńska Marzena, Cieślak-Golonka Maria

2010

Mononuclear copper(II) nitrato complexes with methyl-substituted 4-nitropyridine N-oxide : physicochemical and cytotoxic characteristics.

Puszko Aniela, Krojcer A., Pełczyńska Marzena, Wietrzyk Joanna, Cieślak-Golonka Maria, Jezierska Julia, Adach Anna, Kubiak Maria