Repozytorium

Cooperative Halogen Bonding and π – π Stacking Interactions as Drivers of Polymorphism

Autorzy

Marcin S. Małecki

Marcin Moskwa

Przemysław Dopieralski

Sławomir Szafert

Rok wydania

2025

Czasopismo

ChemPhysChem

Numer woluminu

26

Strony

e202500491/1-e202500491/8

DOI

10.1002/cphc.202500491

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Understanding the mechanisms underlying the formation of different polymorphic forms of a given compound is a fundamental issue in modern physical chemistry, with significant implications for the design of functional materials, including those with pharmaceutical relevance. In the present study, the formation of two polymorphic forms of a polyyne compound is elucidated, as confirmed by X-ray crystallographic analysis. The emergence of these polymorphs results from a delicate interplay between halogen bonding and a network of noncovalent ππ stacking interactions. A combination of experimental techniques, single-crystal X-ray diffraction, and theoretical studies allows us to construct a coherent model that rationalizes the formation of both polymorphic modifications of the investigated system.

Słowa kluczowe

1-haloalkynes, halogen bonds, noncovalent interactions, polymorphs, solid states

Adres publiczny

http://dx.doi.org/10.1002/cphc.202500491

Strona internetowa wydawcy

onlinelibrary.wiley.com

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