Repozytorium

Hydration of NaHCO3, KHCO3, (HCO3-)2, HCO3- and CO32- from molecular dynamics simulation and speed of sound measurements.

Autorzy

Przemysław D. Dopieralski

Andrzej Burakowski

Zdzisław Latajka

Ivar Olovsson

Rok wydania

2011

Czasopismo

Chemical Physics Letters

Numer woluminu

507

Strony

89-95

DOI

10.1016/j.cplett.2011.03.065

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Car–Parrinello molecular dynamics and acoustic method have been applied to determine the hydration of and ions in aqueous solution. From CPMD simulations the hydration numbers are 5.3 and 8.5 for the and ions, respectively. From speed of sound and density measurements the hydration numbers for and are 5.5 and 10.2, respectively. Our attempt to answer the old question concerning the status of in solution quite well support the earlier spectroscopic results that no ()2 is present in the solution but the existence of the minor amount of dimers cannot be definitely excluded.

Adres publiczny

https://doi.org/10.1016/j.cplett.2011.03.065

Strona internetowa wydawcy

http://www.elsevier.com

Podobne publikacje