Repozytorium

Tungsten-catalyzed alkyne metatheses in transition-metal coordination spheres: versatile new syntheses of metallamacrocycles.

Autorzy

Eike B. Bauer

Sławomir Szafert

Frank A. Hampel

John A. Gladysz

Rok wydania

2003

Czasopismo

Organometallics

Numer woluminu

22

Strony

2184-2186

DOI

10.1021/om030195u

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The title reaction (10−15 mol % of (t-BuO)3W(⋮C-t-Bu), chlorobenzene, 80 °C) is applied to octahedral and square-planar 18- and 16-valence-electron rhenium, ruthenium, and platinum complexes with cis- or trans-Ph2P(CH2)6C⋮CCH3 ligands. NMR analyses show ca. 90−70% educt conversions, and 17-membered diphosphine chelates have been isolated in 59−47% yields and crystallographically characterized.

Adres publiczny

https://doi.org/10.1021/om030195u

Strona internetowa wydawcy

https://www.acs.org/content/acs/en.html

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Olefin metatheses in metal coordination spheres: versatile new strategies for the construction of novel monohapto or polyhapto cyclic, macrocyclic, polymacrocyclic, and bridging ligands.

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