Repozytorium

X-ray and electrochemical characterization of high-spin cobalt(II) triazene-1-oxide complexes. Molecular structure of bis[3-(2-methoxyphenyl)-1-ethyltriazen-1-olato]cobalt(II).

Autorzy

Mikołaj F. Rudolf

Zbigniew Ciunik

Kazimierz Gatner

Juliusz A. Wolny

Rok wydania

1992

Czasopismo

Polyhedron

Numer woluminu

11

Strony

2591-2597

DOI

10.1016/S0277-5387(00)80227-2

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The X-ray crystal structure of the title compound was determined. The complex displays strongly distorted octahedral geometry with weak bonds between the methoxy group oxygens and the central ion. The related complex with ortho-chlorine substituted ligands was shown to undergo conversion to the low-spin, square-planar isomer upon doping to the lattice of its nickel(II) analogue. Cyclic voltammery measurements showed that the oxidation potentials of the high-spin, pseudo-octahedral cobalt(II) complexes of triazene-l-oxides are ca 0.1–0.2 V higher than those found for low-spin, square-planar cobalt(II) bis-chelates thereof.

Adres publiczny

https://doi.org/10.1016/S0277-5387(00)80227-2

Strona internetowa wydawcy

http://www.elsevier.com

Podobne publikacje
1993

Cobalt(II) triazene 1-oxide bis(chelates) : a case of planar (low spin) - tetrahedral (high spin) isomerism.

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1992

Remarks on the ground state of low-spin cobalt(II) triazene-1-oxide complexes.

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