Repozytorium

Unusual loss of substituents in the course of cyclization of tetrahydrobilines to dihydroporphyrins.

Autorzy

Jan-Erik Damke

Lechosław Latos-Grażyński

Franz-Peter Montforts

Rok wydania

2008

Czasopismo

Helvetica Chimica Acta

Numer woluminu

91

Strony

177-186

DOI

10.1002/hlca.200890023

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Metallo-tetrahydrobiline rac-8 was prepared to investigate its cyclization directed to the formation of N-confused chlorins. To achieve the site-directed selectivity of the cyclization, the 2-position of rac-2 was activated by an electron-withdrawing cyano function and its 1-position was blocked by a methyl group. In spite of this provision, the cyclization occurred at the apparently blocked 1-position with loss or migration of the methyl substituent.

Adres publiczny

https://doi.org/10.1002/hlca.200890023

Strona internetowa wydawcy

onlinelibrary.wiley.com

Podobne publikacje
2011

Unusual oxidation in the course of synthesis of N-confused nickel tetrahydrobilins.

Damke Jan-Erik, König T., Haake G., Latos-Grażyński Lechosław, Montforts Franz-Peter

2010

New substituents for the stabilization of low-coordinate germanium species: use in access to diazogermylenes.

Brusylovets Oleksii A., Vinichenko O. V., Brusilovets A. I., Lis Tadeusz, Bonnefille E., Mazières S., Couret C.

2014

The unusual binding mechanism of Cu(II) ions to the poly-histidyl domain of a peptide found in the venom of an African viper.

Pontecchiani Fabio, Simonovsky Eyal, Wieczorek Robert, Barbosa Nuno A., Rowińska-Żyrek Magdalena, Potocki Sławomir, Remelli Maurizio, Miller Yifat, Kozłowski Henryk