Repozytorium

Direct synthesis of linear trinuclear M2II MnII complexes with acetate and N—N donor ligands.

Autorzy

Oksana V. Nahorna

Valeriya G. Makhankova

Vladimir N. Kokozay

Irina V. Omelchenko

Viktoriya V. Dyakonenko

Oleg V. Shishkin

Julia Jezierska

Rok wydania

2013

Czasopismo

Journal of Molecular Structure

Numer woluminu

1038

Strony

211-215

DOI

10.1016/j.molstruc.2013.01.048

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Two novel heterometallic complexes with general formula [M2Mn(OAc)6L2], where M = Cd (1), Cu (2) and L = 2,2'-bipyridyl (bpy) for (1), 1,10-phenanthroline (phen) for (2), were obtained using "direct synthesis" approach. Trinuclear molecular structure of the complexes was determined by single crystal X-ray analysis. EPR studies of 2 indicate that the coordination environment in Cu(II) equatorial plane remains unchanged in solution as compared to the initial compound. Due to low volatility of phen the products of its decomposition probably remain on the surface of metal oxides and, therefore, in contrary to previously studied bpy-containing complexes, the compounds with phen are not suitable precursors for binary oxides preparation.

Słowa kluczowe

manganese, Direct synthesis, crystal structure, EPR study, Thermal analysis

Adres publiczny

http://dx.doi.org/10.1016/j.molstruc.2013.01.048

Strona internetowa wydawcy

http://www.elsevier.com

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