Repozytorium

Lactones 31. Synthetic odoriferous unsaturated γ -lactones.

Autorzy

R. Obara

Antoni Szumny

Alicja Wzorek

M. Szmigiel-Pieczewska

Agata Białońska

Zbigniew Ciunik

Czesław Wawrzeńczyk

Rok wydania

2008

Czasopismo

Flavour and Fragrance Journal

Numer woluminu

23

Strony

416-425

DOI

10.1002/ffj.1894

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Starting from g, d-unsaturated terpenoid acids, the corresponding d-iodo-g-lactones and g-iodo-d-lactones
were obtained. Dehydrohalogenation of d-iodo-g-lactones with DBU gave unsaturated g-lactones with an exocyclic or alkyl
chain double bond. Both types of double bonds possessed the E con¼guration. The composition of product mixture of
dehydrohalogenation strongly depended on the conditions (solvent, temperature) of the process. Odour evaluation of the
lactones obtained showed that lactones with two double bonds in the molecule (11 and 12) possess intensive, well-marked,
fresh mushroom odours. Lactones with one double bond and one methyl group at C-4 (5a, 6a, 6b and 5d, 6d, 6e) are char-
acterized, in general, by milky, coconut and creamy odours with different notes. Lactones with two methyl groups at C-4
possess herbal (5c, 5f) or woody (6c) odours.

Słowa kluczowe

iodolactonization, DBU, elimination, lactones, odour analysis, mushroom odour

Adres publiczny

https://doi.org/10.1002/ffj.1894

Strona internetowa wydawcy

onlinelibrary.wiley.com

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