Repozytorium

Sulfonic acid-functionalized silica-coated magnetic nanoparticles as a reusable catalyst for the preparation of pyrrolidinone derivatives under eco-friendly conditions.

Autorzy

Zahra Hosseinzadeh

Ali Ramazani

Hamideh Ahankar

Katarzyna Ślepokura

Tadeusz Lis

Rok wydania

2019

Czasopismo

Silicon

Numer woluminu

11

Strony

2933-2943

DOI

10.1007/s12633-019-0087-2

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The surface of silica-coated CoFe2O4 magnetic nanoparticles (CoFe2O4@SiO2), which is resistant to the oxidation due to silicone coating, was functionalized using chlorosulfonic acid and used as an efficient and recyclable catalyst for the preparation of 3-pyrrolin-2-ones from diethyl acetylenedicarboxylate, an aldehyde and aniline in ethanol solvent at 60 °C. In the presented study, some fascinating chracteritics of such catalyst, such as magnetically separable, simple workup and obtaining a high purity of products by simple recrystallization, have been successfully obtained. The structural features of CoFe2O4@SiO2-SO3H catalyst were elucidated by X-ray powder diffraction (XRPD), thermo-gravimetric studying (TGA), scanning electron microscopy (SEM) and FT-IR spectra.

Słowa kluczowe

Cobalt ferrite, Silica-coated, Sulfonic acid-functionalized, Reusable catalyst, Magnetic nanoparticles, 3-pyrrolin-2-ones

Adres publiczny

http://dx.doi.org/10.1007/s12633-019-0087-2

Strona internetowa wydawcy

http://link.springer.com

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