Repozytorium

Vibrational study of the structural phase transitions for the (CH3NH3)3Sb2Br9 (MABA) and (CH3NH3)3Bi2Br9 (MABB) crystals by infrared spectroscopy.

Autorzy

Ryszard Jakubas

Grażyna Bator

Jan Baran

Rok wydania

1993

Czasopismo

Journal of Physics and Chemistry of Solids

Numer woluminu

54

Strony

1065-1072

DOI

10.1016/0022-3697(93)90015-J

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Infrared spectra of polycrystalline (CH3NH3)3Sb2Br9(MABA) and (CH3NH3)Bi2Br9 (MABB) have been studied in the 90–300 K and 13–300 K temperature ranges, respectively. A systematic temperature dependence study of the internal modes has been carried out. The effects of the dynamical state of methylammonium (MA) cations on their vibrational spectra are discussed. In the higher temperature phases the i.r. spectra reflects the isotropic rotation of CH3NH3+ cations. While in lower temperature phases numerous internal modes show splitting due to both non-equivalent cations in the lattice and a distinct change in their motional state

Adres publiczny

https://doi.org/10.1016/0022-3697(93)90015-J

Strona internetowa wydawcy

http://www.elsevier.com

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