Repozytorium

Open Rotaxane Surgery: What Molecular Editing Can Offer to Supramolecular Chemistry?

Autorzy

Jędrzej P. Perdek

Rafał A. Grzelczak

Bartosz Szyszko

Rok wydania

2025

Czasopismo

ChemPlusChem

Numer woluminu

90

Strony

e202500038/1-e202500038/3

DOI

10.1002/cplu.202500038

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The skeletal editing approach represents a paradigm shift in organic synthesis by directly targeting the molecular skeleton instead of relying on often long and complicated series of organic transformations. Recent advancements in nitrogen atom deletion reactions have enabled unprecedented late-stage, precise modifications of bioactive compounds and complex natural products, influencing a seemingly distant field such as supramolecular chemistry. In a recent contribution, the Leigh group demonstrated the extrusion of a nitrogen atom from an axle of a [2]rotaxane, extending the applicability of molecular editing to complex, mechanically interlocked architectures. This highlight seeks to examine the significance of the skeletal editing method in supramolecular chemistry, address its challenges, and offer an outlook on future directions in this emerging field.

Słowa kluczowe

supramolecular chemistry, mechanically interlocked molecules, skeletal editing, rotaxanes

Adres publiczny

http://dx.doi.org/10.1002/cplu.202500038

Strona internetowa wydawcy

onlinelibrary.wiley.com

Podobne publikacje
2025

Multimodal Molecular Motion in the Rotaxanes and Catenanes Incorporating Flexible Calix[n]phyrin Stations

Grzelczak Rafał A., Basak Tymoteusz, Trzaskowski Bartosz, Kinzhybalo Vasyl, Szyszko Bartosz

2009

N-fusion approach in construction of contracted carbaporphyrinoids: formation of N-fused telluraporphyrin.

Pacholska-Dudziak Ewa, Ulatowski Filip, Ciunik Zbigniew, Latos-Grażyński Lechosław