Repozytorium

Crystal structure and molecular stereochemistry of the 1 : 2 adduct of anionic complex, dicyano-(5,10,15,20-tetramesityleneporphinato) iron(II) with bis(triphenylphosphine)nitrogen(1+), I2, CDCl3 solvate{[(CN)2FeII(TMP)][PPN)2 I2 2CDCl3.

Autorzy

Tadeusz J. Bartczak

Stanisław Wołowiec

Lechosław Latos-Grażyński

Rok wydania

1998

Czasopismo

Inorganica Chimica Acta

Numer woluminu

277

Strony

242-246

DOI

10.1016/S0020-1693(97)06156-2

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Treatment of (meso-tetramesityleneporphinato)iron(III) iodide [(TMP)Fel] with four-fold excess equivalents of bis(triphenyl-phosphine)nitrogen(1+) cyanide {[PPN][CN]} in chloroform solution resulted in the reduction of (TMP)FeIII to (TMP)FeIIII to (TMP)FeII and the formation of low-spin bis-cyanide {[(TMP)Fe(CN2)][PPN]2} complex cocrystallized with iodine and solvent molecules. The crystal and molecular structure of the complex was established crystallographically. There are two [(TMP)Fe(CN)2]2− anions in the unit cell (one half per asymmetric unit), four [PPN] cations, four CDCl3 molecules and two disordered I2 molecules (one half per asymmetric unit). The porphyrin macrocylec has crystallographically required symmetry and is planar with the Fe atom lying at 1/2,0,0.

Słowa kluczowe

crystals structures, Ion complexes, Low-spin complexes, Dicyano-porphyrin complexes

Adres publiczny

https://doi.org/10.1016/S0020-1693(97)06156-2

Strona internetowa wydawcy

http://www.elsevier.com

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