Repozytorium

Decoupling of the order-disorder and displacive contributions to the phase transition in NH4H(ClH2CCOO)2.

Autorzy

M. Zdanowska-Frączek

Ryszard Jakubas

P. Czarnecki

Rok wydania

2005

Czasopismo

Journal of Physics and Chemistry of Solids

Numer woluminu

66

Strony

845-850

DOI

10.1016/j.jpcs.2004.11.003

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The effects of hydrostatic pressure and substitution of Rb+for the ammonium cations on the ferroelectric phase transition temperature in NH4H(ClH2CCOO)2 have been studied by electric permittivity measurements. The transition temperature (Tc) decreases with increasing pressure up to 800 MPa and the pressure coefficient dTc/dp=−1.4×10−2 [K/MPa] has been experimentally determined. The substitution of Rb+ for the ammonium cations has been shown to considerably lower the ferroelectric phase transition temperature Tc. In mixed crystals, additional electric permittivity anomaly has been clearly evidenced. The results are discussed assuming a model, which combines polarizability effects, related to the heavy ion units, with the pseudo-spin tunnelling.

Słowa kluczowe

C. High pressure, D. Ferroelectricity, D. Phase transitions

Adres publiczny

https://doi.org/10.1016/j.jpcs.2004.11.003

Strona internetowa wydawcy

http://www.elsevier.com

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