Repozytorium

Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI2 and D2O.

Autorzy

Hengzhao Li

Mengqi Peng

Zemin Lai

Lei Ning

Xingyue Chen

Xiaoxu Zhang

Pengjie Wang

Roman Szostak

Michal Szostak

Jie An

Rok wydania

2021

Czasopismo

Chemical Communications

Numer woluminu

57

Strony

5195-5198

DOI

10.1039/d1cc01381e

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

A highly chemoselective reductive deuteration of acyl fluorides to provide α,α-dideuterio alcohols with exquisite levels of deuterium incorporation was developed using SmI2 and D2O as the deuterium source. This method introduces acyl fluorides as attractive radical precursors for the generation of reactive acyl-type fluoride ketyls that should find widespread application in many synthetic strategies involving single electron transfer processes.

Adres publiczny

http://dx.doi.org/10.1039/d1cc01381e

Strona internetowa wydawcy

https://www.rsc.org/

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