Repozytorium

Internal rotation in ortho-chloro-substituted biphenyls. Ab initio and molecular dynamics study.

Autorzy

Andrzej Szymoszek

Aleksander Koll

Rok wydania

2003

Czasopismo

Chemical Physics Letters

Numer woluminu

373

Strony

591-598

DOI

10.1016/S0009-2614(03)00663-8

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Structure of the ortho-Cl-substituted biphenyls is studied in vacuo and in the CCl4 solution, by molecular modelling methods. Ab initio determinations of rotational potentials are followed by molecular dynamics simulations, in order to estimate effects of the solvent on conformations. The solvent flattening effect is correlated to molecular volume changes during rotation around the C–C bond. It is concluded, that solvent induced change of rotational barrier can have influence on molecular properties of studied compounds, especially their toxicity.

Adres publiczny

https://doi.org/10.1016/S0009-2614(03)00663-8

Strona internetowa wydawcy

http://www.elsevier.com

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