Repozytorium

Crystal structure and thermoanalytical study of a cadmium(II) complex with 1-allylimidazole.

Autorzy

S. De Angelis Curtis

Maria Kubiak

K. Kurdziel

S. Materazzi

S. Vecchio

Rok wydania

2010

Czasopismo

Journal of Analytical and Applied Pyrolysis

Numer woluminu

87

Strony

175-179

DOI

10.1016/j.jaap.2009.11.007

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The crystal structure of a cadmium(II) 1-allylimidazole complex ([Cd(1-AIm)3(NO3)2], where 1-Aim = 1-allylimidazole), was characterized by single-crystal X-ray diffraction analysis. Thermogravimetry (TG) coupled with an FTIR unit was used to study the thermal behaviour of the complex. A multi-step decomposition occurred in the complex due to the release of the ligand molecules, followed by oxidation. The final residue at 1073 K was found to be cadmium(II) oxide. The oxidative decomposition pattern of the examined complex initially proposed by the percentage mass loss data was proved by the evolved gas analysis. Finally, a kinetic analysis of the oxidative decomposition steps was made using the Kissinger equation, while the complex nature of the decomposition kinetics was revealed by the isoconversional Ozawa–Flynn–Wall method.

Słowa kluczowe

Cadmium(II) complexes, Imidazole derivatives, crystal structure, TG, DSC, Coupled TG-FTIR, EGA, Decomposition kinetics

Adres publiczny

https://doi.org/10.1016/j.jaap.2009.11.007

Strona internetowa wydawcy

http://www.elsevier.com

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