Repozytorium

Synthesis of Shape-Persistent meta-Arylene-Butadiynylene Macrocycles with a Different Ring Size

Autorzy

Marcin Małecki

Dorota Pawelczyk

Bartłomiej Pigulski

Sławomir Szafert

Nurbey Gulia

Rok wydania

2022

Czasopismo

Synthesis-Stuttgart

Numer woluminu

54

Strony

5281-5290

DOI

10.1055/a-1900-3563

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

A series of meta-phenylene-butadiynylene macrocycles was obtained by homocoupling of terminal bis(ethynyl) precursors using Eglinton conditions. Cyclotetramers and cyclopentamers were isolated from the mixture. However, a hexameric analogue was synthesized using a step-by-step approach. Molecular structures of the resulting macrocycles obtained by X-ray single-crystal analysis manifest conformational diversity, indicating significant flexibility of the meta-arylene-butadiynylene macrocycle conjugated skeleton.

Słowa kluczowe

macrocycles, cross-coupling, Eglinton coupling, butadiynes, shape-persistent macrocycles

Adres publiczny

http://dx.doi.org/10.1055/a-1900-3563

Strona internetowa wydawcy

https://www.thieme.com/

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