Repozytorium

A new mixed-valence CuI/CuII three-dimensional coordination polymer constructed with an N,O-donor ligand generated via solvothermal synthesis: structural features and magnetic properties.

Autorzy

Andrzej Kochel

Małgorzata Hołyńska

Kamil Twaróg

Aneta Jezierska

Jarosław J. Panek

Jacek Wojaczyński

Rok wydania

2022

Czasopismo

Acta Crystallographica Section C: Structural Chemistry

Numer woluminu

C78

Strony

405-413

DOI

10.1107/s2053229622005812

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

A new mixed-valence CuI/CuII three-dimensional coordination polymer, poly[[di­aqua­bis­[μ4-2-(pyra­zin-2-yl)quinoline-4-carboxyl­ato]dicopper(I)copper(II)] bis­(tetra­fluorido­borate)], {[Cu3(C14H8N3O2)2(H2O)2](BF4)2}n, was synthesized and characterized, with 2-(pyra­zin-2-yl)quinoline-4-carb­oxy­lic acid being em­ployed as a linker ligand. The ligand was isolated as its hydro­chloride salt, 4-carb­oxy-2-(pyra­zin-2-yl)quinolin-1-ium chloride dihydrate, C14H10N3O2+·Cl·2H2O. The compounds show luminescence at 550 nm for the ligand and at 565 nm for the polymer at 297 K. The ligand structure was rationalized by means of quantum-chemical calculations, which led to a similar conformation to that determined from X-ray diffraction studies.

Słowa kluczowe

quinoline­carb­oxy­lic acid, quinolinium chloride, photoluminescence, magnetic properties, coordination polymer, crystal structure, quantum–chemical calculations.

Adres publiczny

http://dx.doi.org/10.1107/s2053229622005812

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