Repozytorium

The influence of the OHO angle on the proton valency in inter- and intra-molecular hydrogen bonds.

Autorzy

Irena Majerz

Ivar Olovsson

Rok wydania

2010

Czasopismo

Journal of Molecular Structure

Numer woluminu

968

Strony

48-51

DOI

10.1016/j.molstruc.2010.01.018

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The influence of the OHO angle in the hydrogen bond on the potential-energy surface has been studied. The OHO angle has been artificially changed from 140° to 180° to study the influence of the angle on the location of the energy minimum relative to QMRC, the minimum energy reaction path, and BORC, the bond-order reaction path. In the intermolecular hydrogen bond QMRC and BORC are identical, independent on the OHO angle. The intramolecular hydrogen bond is very sensitive to a change in the OHO angle. The agreement between the theoretical results is confirmed by available experimental neutron data.

Słowa kluczowe

Hydrogen bond, Potential-energy surface, Bond-order reaction path

Adres publiczny

https://doi.org/10.1016/j.molstruc.2010.01.018

Strona internetowa wydawcy

http://www.elsevier.com

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