Repozytorium

Charge-density distribution in sodium bis(4-nitrophenyl)phosphate.

Autorzy

Przemysław Starynowicz

Tadeusz Lis

Rok wydania

2014

Czasopismo

Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials

Numer woluminu

B70

Strony

723-731

DOI

10.1107/S2052520614010439

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

The electron-density distribution in sodium bis(4-nitrophenyl)phosphate has been analyzed using the multipole refinement of X-ray diffraction data and of theoretical density-functional theory (DFT) calculations. The ester P-O bonds are particularly long and their topological parameters (density at the bond critical point, Laplacian) are lower than for other P-O bonds. Some disagreement between the experimental and theoretical charges of atoms constituting the nitro groups has been observed and the possible reasons are discussed. Weak polarization effects produced by sodium cations may be observed within the phosphate fragment; they are more manifest in the case of the nitro groups.

Adres publiczny

http://dx.doi.org/10.1107/S2052520614010439

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