Repozytorium

Phase transition and structure of (C3N2H5)2SbF5 single crystal.

Autorzy

Zbigniew Czapla

Monika K. Krawczyk

Adam Ingram

Olaf Czupiński

Rok wydania

2015

Czasopismo

Journal of Physics and Chemistry of Solids

Numer woluminu

87

Strony

233-237

DOI

10.1016/j.jpcs.2015.08.014

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

New crystal of the formula (C3N2H5)2SbF5 was obtained and characterized with DSC, DTA, TGA, structural and dielectric studies. DSC and dielectric studies revealed a structural phase transition of the first order at 216 K on cooling and 220 K on heating. The entropy of the transition ΔS equal to 11.5 J/mol·K gives evidence that the phase transition is order-disorder type. X-ray studies showed that transition undergoes from orthorhombic phase I with a space group of Pmmn to monoclinic phase II with a space group P21/m. The phase transition is proposed to be ferroelastic type. The molecular mechanism of the phase transition is related to ordering of imidazolium cations in phase II that are disordered in phase I.

Słowa kluczowe

phase transition, crystal structure, Electric permittivity

Adres publiczny

http://dx.doi.org/10.1016/j.jpcs.2015.08.014

Strona internetowa wydawcy

http://www.elsevier.com

Podobne publikacje
2021

Room-temperature ferroelasticity and unusual sequence of phase transitions in the crystal of (N2H5)3[CdCl5].

Krawczyk Monika K., Czapla Zbigniew, Ingram Adam, Kozdraś Andrzej, Lis Tadeusz, Przesławski Janusz

2019