Repozytorium

Synthesis, crystal structure and magnetic properties of a 1D mixed-metal-mixed-ligand Ni(II) / Fe(II) coordination polymer built on the nitroprusside anion.

Autorzy

D. V. Shevchenko

S. R. Petrusenko

Vladimir N. Kokozay

Alina Tomkiewicz

Julia Kłak

Jerzy Mroziński

M. V. Krasovska

Oleg V. Shishkin

Wolfgang Linert

Rok wydania

2007

Czasopismo

Inorganica Chimica Acta

Numer woluminu

360

Strony

2846-2850

DOI

10.1016/j.ica.2007.01.012

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

A new complex [Ni(L)Fe(CN)5NO] · 2H2O (L = 4,6,6-trimethyl-1,9-diamino-3,7-di-aza-nona-3-ene) has been obtained and characterized by means of X-ray crystallographic analysis and magnetochemistry. The Fe(CN)5NO2− anion links to the Ni(L)2+ cation through two bridging cyanide groups in a bent fashion. The intrachain Ni⋯Ni and interchain Ni⋯Ni distances are equal to 9.81(8) and 7.75(1) Å, respectively. The magnetic behaviour of the complex indicates the zero field splitting parameter D higher than 3 cm−1 and the average exchange parameter (intra- and interchain) corresponding to direct Ni–Ni magnetic interaction in the crystal lattice equals ∼−0.2 cm−1.

Słowa kluczowe

Nitroprusside, Heteropolynuclear Ni/Fe complex, Magnetochemistry

Adres publiczny

https://doi.org/10.1016/j.ica.2007.01.012

Strona internetowa wydawcy

http://www.elsevier.com

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