Repozytorium

One- and two-photon-induced isomerization of styryl compounds possessing A-π-A′ structure

Autorzy

Beata Jędrzejewska

Marta Gordel

Janusz Szeremeta

Małgorzata A. Kaczorowska

Marek Józefowicz

Marek Samoć

Rok wydania

2016

Czasopismo

Dyes and Pigments

Numer woluminu

132

Strony

237-247

DOI

10.1016/j.dyepig.2016.05.001

Kolekcja

Naukowa

Język

Angielski

Typ publikacji

Artykuł

Streszczenie

Two styryl compounds with A-π-A′ structure that feature a fixed pyridine ring as an electron acceptor (A) and pyridine or 5,6,7,8-tetrahydroisoquinoline cation as the other acceptor (A′) have been synthesized. Their structures were elucidated by means of NMR and IR spectroscopy. One-photon fluorescence, fluorescence quantum yields and lifetimes were investigated. It was found that both visible (408 nm) and near-infrared (800 nm) light promotes the conversion of the E-isomer of the studied compounds to the Z-isomer. Under the UV irradiation (310 nm) the obtained Z-isomer reverts to the initial form in tens of minutes. The observed inter-conversion was found to be fast and efficient. The trans-to-cis isomerization was followed by decomposition of the compound upon longer than 100 s exposure to light as indicated from mass spectra.

Słowa kluczowe

Styryl dyes, Synthesis, One- and two-photon induced isomerization

Adres publiczny

http://dx.doi.org/10.1016/j.dyepig.2016.05.001

Strona internetowa wydawcy

http://www.elsevier.com

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